Production of narrowband tunable extreme-ultraviolet radiation by noncollinear resonance-enhanced four-wave mixing.

نویسندگان

  • S Hannemann
  • U Hollenstein
  • E J van Duijn
  • W Ubachs
چکیده

Fourier-transform-limited extreme-ultraviolet (XUV) radiation (bandwidth approximately < 300 MHz) tunable around 91 nm is produced by use of two-photon resonance-enhanced four-wave mixing on the Kr resonance at 94 093 cm(-1). Noncollinear phase matching ensures the generation of an XUV sum frequency 2 omega1 + omega2 that can be filtered from auxiliary laser beams and harmonics by an adjustable slit. Application of the generated XUV light is demonstrated in spectroscopic investigations of highly excited states in H2 and N2.

برای دانلود متن کامل این مقاله و بیش از 32 میلیون مقاله دیگر ابتدا ثبت نام کنید

ثبت نام

اگر عضو سایت هستید لطفا وارد حساب کاربری خود شوید

منابع مشابه

Ultrahigh-order wave mixing in noncollinear high harmonic generation.

We show that noncollinear high harmonic generation (HHG) can be fully understood in terms of nonlinear optical wave mixing. We demonstrate this by superposing on the fundamental ω1 field its second harmonic ω2 of variable intensity in a noncollinear geometry. It allows us to identify, by momentum conservation, each field's contribution (n1,n2) to the extreme ultraviolet emission at frequency Ω ...

متن کامل

Sum-Frequency-Generation-Based Laser Sidebands for Tunable Femtosecond Raman Spectroscopy in the Ultraviolet

Femtosecond stimulated Raman spectroscopy (FSRS) is an emerging molecular structural dynamics technique for functional materials characterization typically in the visible to near-IR range. To expand its applications we have developed a versatile FSRS setup in the ultraviolet region. We use the combination of a narrowband, ~400 nm Raman pump from a home-built second harmonic bandwidth compressor...

متن کامل

High-order harmonic generation yielding tunable extreme-ultraviolet radiation of high spectral purity.

Production of extreme-ultraviolet radiation by high-order harmonic generation is demonstrated to yield unprecedented spectral purity of lambda/Delta lambda=2.5 x 10(5) at wavelengths covering the entire range 40-100 nm. Tunability and sub-cm(-1) bandwidth of the harmonics are demonstrated in recordings of the He (1s4p) and Ar (3p(5)3d') resonance lines at 52.2 and 86.6 nm. Frequency shift of th...

متن کامل

Freely designable optical frequency conversion in Raman-resonant four-wave-mixing process

Nonlinear optical processes are governed by the relative-phase relationships among the relevant electromagnetic fields in these processes. In this Report, we describe the physics of arbitrary manipulation of Raman-resonant four-wave-mixing process by artificial control of relative phases. As a typical example, we show freely designable optical-frequency conversions to extreme spectral regions, ...

متن کامل

Unidirectional radiation of widely tunable THz wave using a prism coupler under noncollinear phase matching condition

A widely tunable THz wave has been parametrically generated and reported recently by us utilizing a LiNbO3 crystal with a monolithic grating coupler under a noncollinear phase matching condition. However, the output direction of the THz wave is strongly dependent on the generated frequency due to the nature of noncollinear phase matching, as well as the grating coupler. In this letter, a novel ...

متن کامل

ذخیره در منابع من


  با ذخیره ی این منبع در منابع من، دسترسی به آن را برای استفاده های بعدی آسان تر کنید

برای دانلود متن کامل این مقاله و بیش از 32 میلیون مقاله دیگر ابتدا ثبت نام کنید

ثبت نام

اگر عضو سایت هستید لطفا وارد حساب کاربری خود شوید

عنوان ژورنال:
  • Optics letters

دوره 30 12  شماره 

صفحات  -

تاریخ انتشار 2005